Apophis
Resident Iconoclast
I'd straight up go old-school - hydrogen as my lifting gas, etc. Much cheaper...
Hydrogen isn't that much better of a lifting gas than Helium. Its primary advantage lies in its cost, which is much cheaper than Helium. Also, Hydrogen is much more common and easier to produce than Helium.
As far as lifting ability, Hydrogen isn't significantly better either. First, Hydrogen only exists in its gaseous form as a diatomic molecule. Basically this means as a gas, Hydrogen only occurs as two Hydrogen atoms bonded together; H2. Helium, however, does occur as a singluar atom in its gaseous form. Even though Hydrogen has an atomic weight of just over 1.00 (whereas Helium's atomic weight is about 4.00), because Hydrogen as a gas is always diatomic, its atomic weight is actually 2.00.
Now, static lift is primarily determined by the differential density between the lifting gas, and the surrounding fluid medium (in our case, the atmosphere). Under standard atmospheric temperature and pressure, diatomic Hydrogen has a density of 0.0052 lbs/ft3. Helium under these same conditions has a density of 0.0102 lbs/ft3. Air has a density of 0.07647 lbs/ft3 under standard atmospheric conditions at sea level.
For one cubic foot of Hydrogen, static lift under standard sea level conditions is 0.07647-0.0052 = 0.07127 lbs/ft3 of lift
For one cubic foot of Helium, static lift under standard sea level conditions is 0.07647-0.0102 = 0.06627 lbs/ft3 of lift
So, a 1,000 cubic foot envelope filled with Hydrogen would have just over 71 pounds of lift at sea level standard conditions, and the same 1,000 cubic foot envelope filled with Helium would have just over 66 pounds of static lift under these same conditions.
You can see the difference isn't very significant, certainly even less so when we consider the dangers of using Hydrogen as a lifting gas due to its flammability.
Apologies for the overly verbose explanation, but hopefully this sheds a bit of light on the topic.